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Role of Dibromomalonic Acid in the Photosensitivity of the Ru(bpy)3 2+-Catalyzed Belousov−Zhabotinsky Reaction
Journal article

Role of Dibromomalonic Acid in the Photosensitivity of the Ru(bpy)3 2+-Catalyzed Belousov−Zhabotinsky Reaction

Vladimir K Vanag, Anatol M Zhabotinsky and Irving R Epstein
The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory, Vol.104(35), pp.8207-8215
09/01/2000

Abstract

Anions Organic reactions Addition reactions Electrodes Light
Dibromomalonic acid (Br2MA) oxidizes the photoexcited state of the Ru(bpy)3 2+ complex, producing Br2. Br2MA also reduces Ru(bpy)3 3+, yielding Br-. The first of these reactions has a rate proportional to [H+] and plays an important part in the mechanism of photoinhibition of the Belousov−Zhabotinsky reaction. We propose a reaction mechanism that gives good agreement with the experimental data.

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