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Stereocontrolled carbotitanation of alkynylsilanes
Journal article   Peer reviewed

Stereocontrolled carbotitanation of alkynylsilanes

Barry B Snider and Michael Karras
Journal of organometallic chemistry, Vol.179(3), pp.C37-C41
10/23/1979

Abstract

Carbometalation of alkynylsilanes with titanocene dichloride/dialkylaluminum chloride is stereospecifically cis. The alkenyltitanium intermediate can be stereospecifically protonated by aqueous sodium hydroxide or iodinated. Addition of any Lewis base to the alkenyltitanium intermediate induces decomposition of this intermediate to give an alkene by hydrogen atom abstraction from the medium, with loss of stereochemistry.

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